Thermal noise calibration of functionalized cantilevers for force microscopy: effects of the colloidal probe position

Aubin Archambault, Caroline Crauste-Thibierge and Ludovic Bellon, J. Appl. Phys. 135, 094502 (2024)

Article: doi: 10.1063/5.0189480
Dataset:  doi: 10.5281/zenodo.10102664
Software : doi: 10.5281/zenodo.10103601

Colloidal probes are often used in force microscopy when the geometry of the tip-sample interaction should be well controlled. Their calibration requires the understanding of their mechanical response, which is very sensitive to the details of the force sensor consisting of a cantilever and the attached colloid. We present analytical models to describe the dynamics of the cantilever and its load positioned anywhere along its length. The thermal noise calibration of such probes is then studied from a practical point of view, leading to correction coefficients that can be applied in standard force microscope calibration routines. Experimental measurements of resonance frequencies and thermal noise profiles of raw and loaded cantilevers demonstrate the validity of the approach.

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Role of a capping layer on the crystalline structure of Sn thin films grown at cryogenic temperatures on InSb substrates

A.-H. Chen, C.P. Dempsey, M. Pendharkar, A. Sharma, B. Zhang, S. Tan, L. Bellon, S.M. Frolov, C.J. Palmstrom, E. Bellet-Amalric, and M. Hocevar, Nanotechnology 35 075702

[Article] doi: 10.1088/1361-6528/ad079e
[Data set] doi: 10.5281/zenodo.7581136

Metal deposition with cryogenic cooling is a common technique in the condensed matter community for producing ultra-thin epitaxial superconducting layers on semiconductors. However, a significant challenge arises when these films return to room temperature, as they tend to undergo dewetting. This issue can be mitigated by capping the films with an amorphous layer. In this study, we investigate the influence of different in situ fabricated caps on the structural characteristics of Sn thin films deposited at 80 K on InSb substrates. Regardless of the type of capping, we consistently observe that the films remain smooth upon returning to room temperature and exhibit epitaxy on InSb in the cubic Sn (α-Sn) phase. Notably, we identify a correlation between alumina capping using an electron beam evaporator and an increased presence of tetragonal Sn (β-Sn) grains. This suggests that heating from the alumina source may induce a partial phase transition in the Sn layer. The existence of the β-Sn phase induces superconducting behavior of the films by percolation effect. This study highlights the potential for tailoring the structural properties of cryogenic Sn thin films through in situ capping. This development opens avenues for precise control in the production of superconducting Sn films, facilitating their integration into quantum computing platforms.

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Reliability and operation cost of underdamped memories during cyclic erasures

Salambô Dago, Sergio Ciliberto, Ludovic Bellon, Adv. Phys. Res. 2023 2300074 (2023)

[Article] doi: 10.1002/apxr.202300074
[Dataset] doi: 10.5281/zenodo.8307734

The reliability of fast repeated erasures is studied experimentally and theoretically in a 1-bit underdamped memory. The bit is encoded by the position of a micro-mechanical oscillator whose motion is confined in a double well potential. To contain the energetic cost of fast erasures, we use a resonator with high quality factor Q: the erasure work W is close to Landauer’s bound, even at high speed. The drawback is the rise of the system’s temperature T due to a weak coupling to the environment. Repeated erasures without letting the memory thermalize between operations result in a continuous warming, potentially leading to a thermal noise overcoming the barrier between the potential wells. In such case, the reset operation can fail to reach the targeted logical state. The reliability is characterized by the success rate Rsi after i successive operations. WT and Rsi are studied experimentally as a function of the erasure speed. Above a velocity threshold, T soars while Rsi collapses: the reliability of too fast erasures is low. These experimental results are fully justified by two complementary models. We demonstrate that Q≃10 is optimal to contain energetic costs and maintain high reliability standards for repeated erasures at any speed.

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Accelerating the heat diffusion: Fast thermal relaxation of a microcantilever

Basile Pottier, Carlos Plata, Emmanuel Trizac, David Guéry-Odelin and Ludovic Bellon, Phys. Rev. Applied  19, 034072 (2023)

[Article] doi: 10.1103/PhysRevApplied.19.034072
[Data set] doi: 10.5281/zenodo.7669037

In most systems, thermal diffusion is intrinsically slow with respect to mechanical relaxation. We devise here a generic approach to accelerate the relaxation of the temperature field of a 1D object, in order to beat the mechanical time scales. This approach is applied to a micro-meter sized silicon cantilever, locally heated by a laser beam. A tailored driving protocol for the laser power is derived to reach arbitrarily fast the thermal stationary state. The model is implemented experimentally yielding a significant acceleration of the thermal relaxation, up to a factor 30. An excellent agreement with the theoretical predictions is reported. This strategy allows to reach a thermal steady state significantly faster than the natural mechanical relaxation.

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Linking fluctuation and dissipation in spatially extended out-of-equilibrium systems

Alex Fontana and Ludovic Bellon, Physics. Rev. E 107, 034118 (2023)

[Article] doi: 10.1103/PhysRevE.107.034118
[Data set] doi: 10.5281/zenodo.7640707

For systems in equilibrium at a temperature T, thermal noise and energy damping are related to T through the fluctuation-dissipation theorem (FDT). We study here an extension of the FDT to an out-of-equilibrium steady state: a microcantilever subject to a constant heat flux. The resulting thermal profile in this spatially extended system interplays with the local energy dissipation field to prescribe the amplitude of mechanical fluctuations. Using three samples with different damping profiles (localized or distributed), we probe this approach and experimentally demonstrate the link between fluctuations and dissipation. The thermal noise can therefore be predicted a priori from the measurement of the dissipation as a function of the maximum temperature of the micro-oscillator.

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Harmonic calibration of quadrature phase interferometry

Baptiste Ferrero and Ludovic Bellon, EPL 139, 55002 (2022)

[Article] doi: 10.1209/0295-5075/ac8761
[Data set] doi:10.5281/zenodo.6801118

The two output signals of quadrature phase interferometers allow to benefit both from the high sensitivity of interferometry (working inside a fringe) and from an extended input range (counting fringes). Their calibration to reach a linear output is traditionally performed using Heydemann’s correction, which involves fitting one output versus the other by an ellipse. Here we present two alternative methods based on the linear response of the measurement to a sinusoidal input in time, which enables a direct calibration with an excellent linearity. A ten fold improvement with respect to the usual technique is demonstrated on an optical interferometer measuring the deflection of scanning force microscopy cantilevers.

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Virtual double-well potential for an underdamped oscillator created by a feedback loop

Salambô Dago, Jorge Pereda, Sergio Ciliberto and Ludovic Bellon, J. Stat. Mech. 2022, 053209 (2022)

[Article] doi: 10.1088/1742-5468/ac6d62
[Erratum] doi: 10.1088/1742-5468/acd697
[Dataset] doi: 10.5281/zenodo.6497247

Virtual potentials are a very elegant, precise and flexible tool to manipulate small systems and explore fundamental questions in stochastic thermodynamics. In particular double-well potentials have applications in information processing, such as the demonstration of Landauer’s principle. Nevertheless, virtual double-well potentials had never been implemented in underdamped systems. In this article, we detail how to face the experimental challenge of creating a feedback loop for an underdamped system (evolving at much smaller time scale than its overdamped counterpart), in order to build a tunable virtual double-well potential. To properly describe the system behavior in the feedback trap, we express the commutation time in the double-well for all barrier heights, combining for the first time  Kramer’s description, valid at high barriers, with an adjusted model for lower ones. We show that a small hysteresis or delay of the feedback loop in the commutation between the two wells results in a modified velocity distribution, interpreted as a cooling of the kinetic temperature of the system. We successfully address all issues to create experimentally a virtual potential that is statistically indistinguishable from a physical one, with a tunable barrier height and energy step between the two wells.

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Dynamics of information erasure and extension of Landauer’s bound to fast processes

Salambô Dago and Ludovic Bellon, Phys. Rev. Lett. 128, 070604 (2022)
[Article] doi: 10.1103/PhysRevLett.128.070604
[Dataset] doi: 10.5281/zenodo.4807408

Using a double-well potential as a physical memory, we study with experiments and numerical simulations the energy exchanges during erasure processes, and model quantitatively the cost of fast operation. Within the stochastic thermodynamics framework we find the origins of the overhead to Landauer’s Bound required for fast operations: in the overdamped regime this term mainly comes from the dissipation, while in the underdamped regime it stems from the heating of the memory. Indeed, the system is thermalized with its environment at all time during quasi-static protocols, but for fast ones, the inefficient heat transfer to the thermostat is delayed with respect to the work influx, resulting in a transient temperature rise. The warming, quantitatively described by a comprehensive statistical physics description of the erasure process, is noticeable on both the kinetic and potential energy: they no longer comply with equipartition. The mean work and heat to erase the information therefore increase accordingly. They are both bounded by an effective Landauer’s limit kBTeffln2, where Teff is a weighted average of the actual temperature of the memory during the process.

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PDF of position and speed during a fast erasure process: comparison between a numerical simulation and the ansatz we propose – See article Supp. Mat for details.

Force microscopy cantilevers locally heated in a fluid: Temperature fields and effects on the dynamics

Basile Pottier and Ludovic Bellon, Journal of Applied Physics 130, 124502 (2021)

[Article] doi:10.1063/5.0060911
[Data set] doi:10.5281/zenodo.5346796

Atomic force microscopy cantilevers are often, intentionally or not, heated at their extremity. We describe a model to compute the resulting temperature field in the cantilever and in the surrounding fluid on a wide temperature range. In air and for common geometries, the heat fluxes in the cantilever and to the environment are of comparable magnitude. We then infer how the fluid–structure interaction is modified due to heating and predict the induced changes in the dynamics of the system. In particular, we describe how the resonance frequencies of the cantilever shift with a temperature increase due to two competing processes: softening of the cantilever and decrease of the fluid inertial effects. Our models are illustrated by experiments on a set of cantilevers spanning the relevant geometries to explore the relative importance of both effects.

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Thermal noise of a cryo-cooled silicon cantilever locally heated up to its melting point

Alex Fontana, Richard Pedurand, Vincent Dolique, Ghaouti Hansali, Ludovic Bellon, Physical Review E 103, 062125 (2021)

[Article] doi: 10.1103/PhysRevE.103.062125
[Data set] doi: 10.5281/zenodo.4696489

 The Fluctuation-Dissipation Theorem (FDT) is a powerful tool to estimate the thermal noise of physical systems in equilibrium. In general however, thermal equilibrium is an approximation, or cannot be assumed at all. A more general formulation of the FDT is then needed to describe the behavior of the fluctuations. In our experiment we study a micro-cantilever brought out-ofequilibrium by a strong heat flux generated by the absorption of the light of a laser. While the base is kept at cryogenic temperatures, the tip is heated up to the melting point, thus creating the highest temperature difference the system can sustain. We independently estimate the temperature profile of the cantilever and its mechanical fluctuations, as well as its dissipation. We then demonstrate how the thermal fluctuations of all the observed degrees of freedom, though increasing with the heat flux, are much lower than what is expected from the average temperature of the system. We interpret these results thanks to a minimal extension of the FDT: this dearth of thermal noise arises from a dissipation shared between clamping losses and distributed damping.

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